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Gold-Catalyzed Rearrangement of Propargyl Alcohols Using Coupling Constants to Determine Isomeric Ratios

Title: Gold-Catalyzed Rearrangement of Propargyl Alcohols Using Coupling Constants to Determine Isomeric Ratios
Language: English
Authors: Cheng, Xinpeng; Chen, Jonna; Gainer, Morgan J. (ORCID 0000-0002-4034-687X); Zhang, Liming (ORCID 0000-0002-5306-1515)
Source: Journal of Chemical Education. Oct 2019 96(10):2348-2351.
Availability: Division of Chemical Education, Inc. and ACS Publications Division of the American Chemical Society. 1155 Sixteenth Street NW, Washington, DC 20036. Tel: 800-227-5558; Tel: 202-872-4600; e-mail: eic@jce.acs.org; Web site: http://pubs.acs.org/jchemeduc
Peer Reviewed: Y
Page Count: 4
Publication Date: 2019
Document Type: Journal Articles; Reports - Descriptive
Education Level: Higher Education; Postsecondary Education
Descriptors: Organic Chemistry; Synthesis; College Science; Science Instruction; Science Experiments; Metallurgy; Spectroscopy
DOI: 10.1021/acs.jchemed.9b00007
ISSN: 0021-9584
Abstract: Gold is an increasingly prominent transition metal in organic synthesis. The air-stable, water-insensitive cationic gold(I) catalysts enable varieties of synthetic transformations with a simple reaction setup. However, this increased importance has not coincided with an increase in the application of gold in second-year organic chemistry courses. An experiment is described that includes a gold-catalyzed rearrangement of propargyl alcohols targeted at second-year organic chemistry students. The reaction produces a mixture of "E" and "Z" isomers of an enone product that students analyze by [superscript 1]H NMR spectroscopy to determine the major product.
Abstractor: As Provided
Entry Date: 2019
Accession Number: EJ1231343
Database: ERIC