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Ecofriendly Synthesis of DHPMs using Copper-based Nano catalysts and Evaluation of Antibacterial Activity

Title: Ecofriendly Synthesis of DHPMs using Copper-based Nano catalysts and Evaluation of Antibacterial Activity
Authors: Sharma, Khushboo; Khatik, Narsingh; Khandelwal, Abhinav Raj; Meena, Ravina; Bhadauria, Seema; Singh, Malvika; Sachdeva, Harshita
Source: Croatica Chemica Acta ; ISSN 1334-417X (Online) ; ISSN 0011-1643 (Print) ; ISSN-L 0011-1643 ; CODEN CCACAA ; Volume 96 ; Issue 2
Publisher Information: Croatian Chemical Society
Publication Year: 2023
Collection: Hrčak - Portal of scientific journals of Croatia / Portal znanstvenih časopisa Republike Hrvatske
Subject Terms: CuFe2O4 NPs; CuO-CeO2 NC; green synthesis; Biginelli compounds; microwave irradiation
Description: A new catalytic approach has been developed under microwave irradiation for the multicomponent reaction (MCR) of aromatic aldehydes, urea/thiourea and ethylacetoacetate to give corresponding dihydropyrimidinones (DHPMs) by using CuFe2O4/CuO-CeO2 nanoparticles (NPs) as heterogeneous and recyclable catalysts. 3, 4-Dihydropyrimidin-2(1H) ones/thiones are synthesized in higher yields (80-95 %) and short reaction time (8−10 minutes) at 245 Watts. It is applicable for both types of aromatic aldehydes containing EWS as well as EDS. Further, the synthesized compounds were evaluated for antibacterial activity against E. coli, B. subtilis, B. megaterium, and P. vulgaris. Among the compounds tested, ethyl-6-methyl-2-oxo-4-(4-chlorophenyl)-1,2,3,4-tetrahydropyrimidin-5-carboxylate, 4c showed response against B. subtilis, B. megaterium, and P. vulgaris and ethyl-6-methyl-2-oxo-4-(4-fluorophenyl)-1,2,3,4-tetrahydropyrimidin-5-carboxylate, 4h showed –ve response against E. coli, B. subtilis, B. megaterium, and P. vulgaris.
Document Type: article in journal/newspaper
File Description: application/pdf
Language: English
Relation: https://doi.org/10.5562/cca4001; https://hrcak.srce.hr/308894
DOI: 10.5562/cca4001
Availability: https://doi.org/10.5562/cca4001; https://hrcak.srce.hr/308894; https://hrcak.srce.hr/file/445874
Rights: info:eu-repo/semantics/openAccess ; Croatica Chemica Acta is at the highest possible level of Open Access, meaning that all content is immediately and freely available to anyone, anywhere, to be downloaded, printed, distributed, read, reused, self archived, and re-mixed (including commercially) without restriction, as long as the author and the original source are properly at-tributed according to the Creative Commons Attribution 4.0 International License (CC BY). The author(s) hold the copyright and retain publishing rights without restrictions. CC BY (Creative Commons Attribution) is the most accommodating of public copyright licenses as defined by Creative Commons, a nonprofit organization that provides legal tools for sharing and use of creative works and research. The CC BY license is recommended for maximum dissemination and use of licensed materials. All content published in Croatica Chemica Acta is available under CC BY, meaning anyone is free to use and reuse the content provided the original source and authors are credited. The copyright is held and retained. The author(s) hold the copyright without restrictions. CC BY is the appropriate license for publicly funded research; it maximizes the potential for both economic and scholarly impact, protects the rights of authors and strengthens the long-standing tradition of appropriate attribution and credit for scholarship.
Accession Number: edsbas.103FAE6F
Database: BASE