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Tunable functional coverage of biocompatible magnesium silicate nanotubes by microwave-assisted silanization

Title: Tunable functional coverage of biocompatible magnesium silicate nanotubes by microwave-assisted silanization
Authors: Secchi, Valeria; D'Alessio, Daniela; Erroi, Andrea; Mostoni, Silvia; Capitani, Giancarlo; Calloni, Alberto; Bussetti, Gianlorenzo; D'Arienzo, Massimiliano; Lorenzi, Roberto; Keinan-Adamsky, Keren; Rahimipour, Shai; Monguzzi, Angelo; Campione, Marcello
Contributors: Secchi, V; D'Alessio, D; Erroi, A; Mostoni, S; Capitani, G; Calloni, A; Bussetti, G; D'Arienzo, M; Lorenzi, R; Keinan-Adamsky, K; Rahimipour, S; Monguzzi, A; Campione, M
Publisher Information: Royal Society of Chemistry; GB
Publication Year: 2025
Collection: Università degli Studi di Milano-Bicocca: BOA (Bicocca Open Archive)
Subject Terms: nanotube; microwave assisted synthesi; silanization; surface characterization
Description: The controlled synthesis of biocompatible nanomaterials with tailored composition, size, and functionalities has driven the advancement of nanomedicine, enabling the development of innovative diagnostic and therapeutic strategies. A key challenge in this field is the design of nano-objects exhibiting multiple functionalities, each dedicated to a specific diagnostic or therapeutic purpose. Among these, synthetic stoichiometric chrysotile nanotubes stand out as a highly biocompatible class of non-carbon nanotubes, already demonstrating their potential for diverse applications, including fluorescence, magnetism, singlet-oxygen generation, and scintillation. Expanding this functional versatility, we report a finely tunable approach for controlling the surface silanization using 3-aminopropyl-trimethoxysilane. This is achieved via a microwave-assisted synthesis, which enables mild reaction conditions and significantly reduces processing time. A comprehensive multi-technique characterization is employed to elucidate the structural and chemical features of the mineral-silane interface and the underlying reaction mechanism.
Document Type: article in journal/newspaper
File Description: STAMPA
Language: English
Relation: info:eu-repo/semantics/altIdentifier/pmid/40843488; info:eu-repo/semantics/altIdentifier/wos/WOS:001554766400001; volume:17; issue:35; firstpage:20259; lastpage:20268; numberofpages:10; journal:NANOSCALE; https://hdl.handle.net/10281/565362
DOI: 10.1039/d5nr02385h
Availability: https://hdl.handle.net/10281/565362; https://doi.org/10.1039/d5nr02385h
Rights: info:eu-repo/semantics/openAccess ; license:Creative Commons ; license uri:http://creativecommons.org/licenses/by-nc/4.0/
Accession Number: edsbas.1A9B7E2D
Database: BASE