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Vertical and horizontal variability and representativeness of the water vapor isotope composition in the lower troposphere: insight from Ultralight Aircraft flights in southern France during summer 2021

Title: Vertical and horizontal variability and representativeness of the water vapor isotope composition in the lower troposphere: insight from Ultralight Aircraft flights in southern France during summer 2021
Authors: Zannoni, Daniele; Steen-Larsen, Hans, Christian; Sodemann, Harald; Thurnherr, Iris; Flamant, Cyrille; Chazette, Patrick; Totems, Julien; Werner, Martin; Raybaut, Myriam
Contributors: Geophysical Institute Bergen (GFI / BiU); University of Bergen (UiB); Department of Environmental Sciences, Informatics and Statistics Venezia; University of Ca’ Foscari Venice, Italy; Institute for Atmospheric and Climate Science Zürich (IAC); Eidgenössische Technische Hochschule - Swiss Federal Institute of Technology Zürich (ETH Zürich); ATMOSPHERE - LATMOS; Laboratoire Atmosphères, Observations Spatiales (LATMOS); Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Institut national des sciences de l'Univers (INSU - CNRS)-Sorbonne Université (SU)-Centre National de la Recherche Scientifique (CNRS)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Institut national des sciences de l'Univers (INSU - CNRS)-Sorbonne Université (SU)-Centre National de la Recherche Scientifique (CNRS); Laboratoire des Sciences du Climat et de l'Environnement Gif-sur-Yvette (LSCE); Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)-Direction de Recherche Fondamentale (CEA) (DRF (CEA)); Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA); Chimie Atmosphérique Expérimentale (CAE); Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)-Direction de Recherche Fondamentale (CEA) (DRF (CEA)); Alfred-Wegener-Institut, Helmholtz-Zentrum für Polar- und Meeresforschung = Alfred Wegener Institute for Polar and Marine Research = Institut Alfred-Wegener pour la recherche polaire et marine (AWI); Helmholtz-Gemeinschaft = Helmholtz Association; DPHY, ONERA, Université Paris Saclay Palaiseau; ONERA-Université Paris-Saclay; European Project: 821868,H2020-SPACE-2018-2020,H2020-SPACE-2018,LEMON(2019)
Source: https://hal.science/hal-04884602 ; 2025.
Publisher Information: CCSD
Publication Year: 2025
Collection: HAL-CEA (Commissariat à l'énergie atomique et aux énergies alternatives)
Subject Terms: [SDU.OCEAN]Sciences of the Universe [physics]/Ocean; Atmosphere
Description: International audience ; The isotopic composition of water vapor is a valuable tool to track atmospheric hydrological processes and to evaluate numerical models simulating the water cycle. To ensure accurate model-observation comparisons, understanding the spatial and temporal distribution of water vapor isotopes in the troposphere is crucial. The challenging task of obtaining highly resolved water vapor isotopic observations is typically addressed through airborne measurements performed onboard conventional aircrafts, but these offer limited microscale insights. This study utilizes observations from ultralight aircraft to examine the water vapor isotopic composition in the lower troposphere of southern France during late summer 2021. By combining the observations with conceptual and numerical models, we identify the main processes driving vertical and spatial variability of isotopic composition and we highlight the detection of short-lived, small-scale processes. The key findings of this study are that (i) at the hourly and sub-daily scales, vertical mixing is the dominant process affecting isotopic variability in the lowermost troposphere and boundary layer above the study site; (ii) evapotranspiration significantly impacts the water vapor isotopic signature, as revealed by the δ18O-δD relationship; (iii) measurable structures of the water isotopic fields emerge on the scale of 100s of m. The latter are particularly evident for δD, which also exhibit the largest differences in horizontal and vertical gradients. When combined with other airborne datasets, our results support a simple model forced with surface observations to simulate the vertical distribution of tropospheric δD, enhancing the comparison between surface observations and satellite data.
Document Type: report
Language: English
Relation: https://doi.org/10.5281/zenodo.7864006; info:eu-repo/grantAgreement//821868/EU/Lidar Emitter and Multispecies greenhouse gases Observation iNstrument/LEMON
DOI: 10.5194/egusphere-2024-3394
Availability: https://hal.science/hal-04884602; https://hal.science/hal-04884602v1/document; https://hal.science/hal-04884602v1/file/egusphere-2024-3394.pdf; https://doi.org/10.5194/egusphere-2024-3394
Rights: http://creativecommons.org/licenses/by/ ; info:eu-repo/semantics/OpenAccess
Accession Number: edsbas.29CC62CC
Database: BASE