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Linear‐Dendritic Alternating Copolymers

Title: Linear‐Dendritic Alternating Copolymers
Authors: Sun, Haotian; Haque, Farihah M.; Zhang, Yi; Commisso, Alex; Mohamed, Mohamed Alaa; Tsianou, Marina; Cui, Honggang; Grayson, Scott M.; Cheng, Chong
Contributors: National Science Foundation
Source: Angewandte Chemie ; volume 131, issue 31, page 10682-10686 ; ISSN 0044-8249 1521-3757
Publisher Information: Wiley
Publication Year: 2019
Collection: Wiley Online Library (Open Access Articles via Crossref)
Description: Herein, the design, synthesis, and characterization of an unprecedented copolymer consisting of alternating linear and dendritic segments is described. First, a 4th‐generation Hawker‐type dendron with two azide groups was synthesized, followed by a step‐growth azide‐alkyne “click” reaction between the 4th‐generation diazido dendron and poly(ethylene glycol) diacetylene to create the target polymers. Unequal reactivity of the functional groups was observed in the step‐growth polymerization. The resulting copolymers, with alternating hydrophilic linear and hydrophobic dendritic segments, can spontaneously associate into a unique type of microphase‐segregated nanorods in water.
Document Type: article in journal/newspaper
Language: English
DOI: 10.1002/ange.201903402
Availability: https://doi.org/10.1002/ange.201903402; https://api.wiley.com/onlinelibrary/tdm/v1/articles/10.1002%2Fange.201903402; https://onlinelibrary.wiley.com/doi/pdf/10.1002/ange.201903402; https://onlinelibrary.wiley.com/doi/full-xml/10.1002/ange.201903402; https://onlinelibrary.wiley.com/doi/am-pdf/10.1002/ange.201903402
Rights: http://onlinelibrary.wiley.com/termsAndConditions#am ; http://onlinelibrary.wiley.com/termsAndConditions#vor
Accession Number: edsbas.2D1D1875
Database: BASE