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Dicarboxylic acids as pH sensors for hyperpolarized 13 C magnetic resonance spectroscopic imaging

Title: Dicarboxylic acids as pH sensors for hyperpolarized 13 C magnetic resonance spectroscopic imaging
Authors: Korenchan, DE; Taglang, C; von Morze, C; Blecha, JE; Gordon, JW; Sriram, R; Larson, PEZ; Vigneron, DB; VanBrocklin, HF; Kurhanewicz, J; Wilson, DM; Flavell, RR
Source: Analyst, vol 142, iss 9
Publisher Information: eScholarship, University of California
Publication Year: 2017
Collection: University of California: eScholarship
Subject Terms: 3402 Inorganic Chemistry (for-2020); 34 Chemical Sciences (for-2020); Bioengineering (rcdc); Biomedical Imaging (rcdc); Carbon Isotopes (mesh); Dicarboxylic Acids (mesh); Hydrogen-Ion Concentration (mesh); Magnetic Resonance Imaging (mesh); Magnetic Resonance Spectroscopy (mesh); Phantoms; Imaging (mesh); 0301 Analytical Chemistry (for); 0399 Other Chemical Sciences (for); Analytical Chemistry (science-metrix); 3401 Analytical chemistry (for-2020)
Time: 1429 - 1433
Description: Imaging tumoral pH may help to characterize aggressiveness, metastasis, and therapeutic response. We report the development of hyperpolarized [2-13C,D10]diethylmalonic acid, which exhibits a large pH-dependent 13C chemical shift over the physiological range. We demonstrate that co-polarization with [1-13C,D9]tert-butanol accurately measures pH via13C NMR and magnetic resonance spectroscopic imaging in phantoms.
Document Type: article in journal/newspaper
File Description: application/pdf
Language: unknown
Relation: qt1hc2h13n; https://escholarship.org/uc/item/1hc2h13n; https://escholarship.org/content/qt1hc2h13n/qt1hc2h13n.pdf
DOI: 10.1039/c7an00076f
Availability: https://escholarship.org/uc/item/1hc2h13n; https://escholarship.org/content/qt1hc2h13n/qt1hc2h13n.pdf; https://doi.org/10.1039/c7an00076f
Rights: public
Accession Number: edsbas.313D8B4
Database: BASE