| Title: |
Molecular Engineering of Interlayer Exciton Delocalization in 2D Perovskites |
| Authors: |
Boeije, Yorrick; Lie, Fabian; Dubajić, Miloš; GARIP, Ediz; MAUFORT, Arthur; Biega, Raisa-Iona; LENAERS, Stijn; Sauty, Mylène; Ghosh, Pratyush; Radić, Aleksandar; Loher, Amélie; La Magna, Paola; Salway, Hayden; Ashoka, Arjun; Chua, Xian Wei; Gu, Qichun; Van Hecke, Kristof; LUTSEN, Laurence; VANDERZANDE, Dirk; Rao, Akshay; VAN GOMPEL, Wouter; Leppert, Linn; Stranks, Samuel D. |
| Contributors: |
Boeije, Yorrick; Lie, Fabian; Dubajić, Miloš; GARIP, Ediz; MAUFORT, Arthur; Biega, Raisa-Iona; LENAERS, Stijn; Sauty, Mylène; Ghosh, Pratyush; Radić, Aleksandar; Loher, Amélie; La Magna, Paola; Salway, Hayden; Ashoka, Arjun; Chua, Xian Wei; Gu, Qichun; Van Hecke, Kristof; LUTSEN, Laurence; VANDERZANDE, Dirk; Rao, Akshay; VAN GOMPEL, Wouter; Leppert, Linn; Stranks, Samuel D. |
| Publication Year: |
2025 |
| Collection: |
Document Server@UHasselt (Universiteit Hasselt) |
| Description: |
In recent years, significant progress has been made in improving the stability, photocurrent efficiency and charge transport properties of 2D hybrid perovskites, making them increasingly relevant for optoelectronic devices. Although these layered systems are typically considered quantum wells due to carrier confinement, an emerging strategy is to generate new perovskite functionalities with -conjugated electroactive cores as spacer molecules, which introduce ; Y.B. acknowledges the Winton Programme for Physics of Sustainability for funding. F.K.L and Li.L. acknowledge f inancial support by the Dutch Research Council (NWO) through a Vidi grant (grant number VI.Vidi.223.072). This research used resources of the Oak Ridge Leadership Computing Facility, which is a U.S. Department of Energy Office (U.S. DOE) Science User Facility supported under Contract DE-AC05−00OR22725 (accessed through the INCITE program). We also acknowledge computational resources on the supercomputer Snellius provided through the NWO Domain Science. S.D.S. acknowledges the Royal Society and Tata Group (grant no. UF150033, URF\R \221026). M.D. acknowledges UKRI guarantee funding for Marie Sklodowska-Curie Actions Postdoctoral Fellowships 2022 (EP/Y024648/1). La.L., D.V., S.L., and W.T.M.V.G. thank the FWO for the funding of the FWO-SBO project PROCEED (S002019N). K.V.H., P.L.M., La.L., D.V., and W.T.M.V.G. are grateful to the FWO for the funding of the senior FWO research projects G043320N and G0A8723N. A.M. acknowledges the FWO for funding his FWO fundamental research PhD grant (1115721N). E.G. is funded by the special research fund (BOF) of Hasselt University under grant BOF23OWB24. X.W.C. thanks the Agency for Science, Technology and Research (A*STAR, Singapore) for the National Science Scholarship. A. L. acknowledges the Cambridge Trust for funding. The authors acknowledge the European Research Council (ERC) under the European Union’s Horizon Europe research and innovation program (VAPOURISE, grant agreement No. 101169608). |
| Document Type: |
article in journal/newspaper |
| File Description: |
application/pdf |
| Language: |
English |
| Relation: |
This article is licensed under CC-BY 4.0; Journal of the American Chemical Society; https://hdl.handle.net/1942/46690; 31557; 35; 31541; 147; 001555722200001 |
| DOI: |
10.1021/jacs.5c05621 |
| Availability: |
https://hdl.handle.net/1942/46690; https://doi.org/10.1021/jacs.5c05621 |
| Rights: |
info:eu-repo/semantics/openAccess |
| Accession Number: |
edsbas.450F42E |
| Database: |
BASE |