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Low-temperature magnetic crossover in the topological kagome magnet TbMn6Sn6

Title: Low-temperature magnetic crossover in the topological kagome magnet TbMn6Sn6
Authors: Mielke III, C; Ma, WL; Pomjakushin, V; Zaharko, O; Sturniolo, S; Liu, X; Ukleev, V; White, JS; Yin, J-X; Tsirkin, SS; Larsen, CB; Cochran, TA; Medarde, M; Porée, V; Das, D; Gupta, R; Wang, CN; Chang, J; Wang, ZQ; Khasanov, R; Neupert, T; Amato, A; Liborio, L; Jia, S; Hasan, MZ; Luetkens, H; Guguchia, Z
Source: Communications Physics, vol 5, iss 1
Publisher Information: eScholarship, University of California
Publication Year: 2022
Collection: University of California: eScholarship
Subject Terms: 51 Physical Sciences (for-2020); 5104 Condensed Matter Physics (for-2020); 40 Engineering (for-2020); 49 Mathematical sciences (for-2020)
Description: Magnetic topological phases of quantum matter are an emerging frontier in physics and materials science, of which kagome magnets appear as a highly promising platform. Here, we explore magnetic correlations in the recently identified topological kagome system TbMn6Sn6 using muon spin rotation, combined with local field analysis and neutron diffraction. Our studies identify an out-of-plane ferrimagnetic structure with slow magnetic fluctuations which exhibit a critical slowing down below TC1*$${T}_{{{{{{{{\rm{C1}}}}}}}}}^{* }$$ ≃ 120 K and finally freeze into static patches with ideal out-of-plane order below TC1 ≃ 20 K. We further show that hydrostatic pressure of 2.1 GPa stabilises the static out-of-plane topological ferrimagnetic ground state in the whole volume of the sample. Therefore the exciting perspective arises of a magnetically-induced topological system whose magnetism can be controlled through external parameters. The present results will stimulate theoretical investigations to obtain a microscopic understanding of the relation between the low-temperature volume-wise magnetic evolution of the static c-axis ferrimagnetic patches and the topological electronic properties in TbMn6Sn6.
Document Type: article in journal/newspaper
File Description: application/pdf
Language: unknown
Relation: qt3529h2n1; https://escholarship.org/uc/item/3529h2n1; https://escholarship.org/content/qt3529h2n1/qt3529h2n1.pdf
DOI: 10.1038/s42005-022-00885-4
Availability: https://escholarship.org/uc/item/3529h2n1; https://escholarship.org/content/qt3529h2n1/qt3529h2n1.pdf; https://doi.org/10.1038/s42005-022-00885-4
Rights: public
Accession Number: edsbas.45B16CD8
Database: BASE