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Synthesis and characterization of poly[phenyl(fluoroalkyloxaalkane)silanediyl]s

Title: Synthesis and characterization of poly[phenyl(fluoroalkyloxaalkane)silanediyl]s
Authors: Zuev, Vjacheslav V.; Skvortsov, Nikolai K.
Source: Journal of Polymer Science Part A: Polymer Chemistry ; volume 41, issue 23, page 3761-3767 ; ISSN 0887-624X 1099-0518
Publisher Information: Wiley
Publication Year: 2003
Collection: Wiley Online Library (Open Access Articles via Crossref)
Description: Monomeric fluoroalkoxyalkyl(phenyl)dichlorosilanes were synthesized with quantitative yields by hydrosilylation of allyl ethers of fluoroalcohols with phenyldichlorosilane with Pt(Ph 3 Sb) 2 Cl 2 complex as a catalyst. Starting from these monomers, corresponding polysilanes with weight‐average molecular weights of 2–3 × 10 4 were obtained by the Wurtz reaction. Increasing the CF 2 groups containing two to six monomer units caused the char yields to increase from 3 to 48% at 800 °C in air. The emission characteristics of these polysilanes in a chloroform solution were examined. They had a narrow peak at 344 nm with a small Stokes shift (≈20 nm). © 2003 Wiley Periodicals, Inc. J Polym Sci Part A: Polym Chem 41: 3761–3767, 2003
Document Type: article in journal/newspaper
Language: English
DOI: 10.1002/pola.10945
Availability: https://doi.org/10.1002/pola.10945; https://api.wiley.com/onlinelibrary/tdm/v1/articles/10.1002%2Fpola.10945; https://onlinelibrary.wiley.com/doi/pdf/10.1002/pola.10945
Rights: http://onlinelibrary.wiley.com/termsAndConditions#vor
Accession Number: edsbas.74A02DD
Database: BASE