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Modeling Pu-239 Fission Fragment De-Excitation applying the Total Monte Carlo method in TALYS

Title: Modeling Pu-239 Fission Fragment De-Excitation applying the Total Monte Carlo method in TALYS
Authors: Karlsson, Peter; Al-Adili, Ali; Göök, Alf; Gao, Zhihao; Pomp, Stephan; Sjöstrand, Henrik; Solders, Andreas; Koning, Arjan
Publisher Information: Uppsala universitet, Institutionen för fysik och astronomi; Uppsala universitet, Tillämpad kärnfysik; IAEA, Dept Nucl Sci & Applicat, Div Phys & Chem Sci, Nucl Data Sect, POB 100, Vienna, Austria.
Publication Year: 2025
Collection: Uppsala University: Publications (DiVA)
Subject Terms: Subatomic Physics; Subatomär fysik
Description: In this study, we applied the Total Monte Carlo (TMC) methodology in de-excitation simulations of primary fission fragments (FF) using the TALYS code. The goal was to develop and optimise a methodology to benchmark initial fission model assumptions on fission mass yield distributions, excitation energy sharing and angular momentum population. The study was performed on the thermal neutron induced fission of Pu-239(n(th),f). The work aimed at evaluating fission model deficiencies and parameter sensitivities. We systematically varied TALYS input data by generating 5000 random files through the GEF code, randomizing 94 model parameters that affect fission yields and energy distributions within 3% of their default values. This variation revealed significant changes in the fission observables, such as prompt neutron and gamma-ray multiplicities and energy spectra. The results indicate some systematic defects in the assumed excitation-energies and angular momenta. Another outcome from the study is the identification of a need for new correlation measurements on prompt neutrons and gamma-rays from the Pu-239(n(th),f) reaction, as well as an updated evaluation.
Document Type: conference object
File Description: application/pdf
Language: English
Relation: EPJ Web of Conferences, 2100-014X; 7TH INTERNATIONAL WORKSHOP ON COMPOUND-NUCLEAR REACTIONS AND RELATED TOPICS, CNR*24; ISI:001453120000032
DOI: 10.1051/epjconf/202532207005
Availability: http://urn.kb.se/resolve?urn=urn:nbn:se:uu:diva-556713; https://doi.org/10.1051/epjconf/202532207005
Rights: info:eu-repo/semantics/openAccess
Accession Number: edsbas.78E55CE2
Database: BASE