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Heralded initialization of charge state and optical-transition frequency of diamond tin-vacancy centers

Title: Heralded initialization of charge state and optical-transition frequency of diamond tin-vacancy centers
Authors: Brevoord, Julia M.; De Santis, Lorenzo; Yamamoto, Takashi; Pasini, Matteo; Codreanu, Nina; Turan, Tim; Beukers, Hans K.C.; Waas, Christopher; Hanson, Ronald
Contributors: Netherlands Enterprise Agency; Dutch Research Council; European Union’s
Source: Physical Review Applied ; volume 21, issue 5 ; ISSN 2331-7019
Publisher Information: American Physical Society (APS)
Publication Year: 2024
Description: Diamond tin-vacancy centers have emerged as a promising platform for quantum information science and technology. A key challenge for their use in more-complex quantum experiments and scalable applications is the ability to prepare the center in the desired charge state with the optical transition at a predefined frequency. Here we report on heralding such successful preparation using a combination of laser excitation, photon detection, and real-time logic. We first show that fluorescence photon counts collected during an optimized resonant probe pulse strongly correlate with the subsequent charge state and optical-transition frequency, enabling real-time heralding of the desired state through threshold photon counting. We then implement and apply this heralding technique to photoluminescence-excitation measurements, coherent optical driving, and an optical Ramsey experiment, finding strongly increased optical coherence with increasing threshold. Finally, we demonstrate that the prepared optical frequency follows the probe laser across the inhomogeneous linewidth, enabling tuning of the transition frequency over multiple homogeneous linewidths. Published by the American Physical Society 2024
Document Type: article in journal/newspaper
Language: English
DOI: 10.1103/physrevapplied.21.054047
DOI: 10.1103/PhysRevApplied.21.054047
DOI: 10.1103/PhysRevApplied.21.054047/fulltext
Availability: https://doi.org/10.1103/physrevapplied.21.054047; https://link.aps.org/article/10.1103/PhysRevApplied.21.054047; http://harvest.aps.org/v2/journals/articles/10.1103/PhysRevApplied.21.054047/fulltext
Rights: https://creativecommons.org/licenses/by/4.0/
Accession Number: edsbas.893BDB47
Database: BASE