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Laser‐Induced Graphene from Waste Almond Shells

Title: Laser‐Induced Graphene from Waste Almond Shells
Authors: Steksova, Yulia; Bressi, Anna Chiara; Galliani, Marina; Marino, Attilio; Ciofani, Gianni; Machado‐Charry, Eduardo; Bernal, Hilda Gomez; Francini, Alessandra; Sebastiani, Luca; Greco, Francesco
Contributors: Steksova, Yulia; Bressi, Anna Chiara; Galliani, Marina; Marino, Attilio; Ciofani, Gianni; Machado‐charry, Eduardo; Bernal, Hilda Gomez; Francini, Alessandra; Sebastiani, Luca; Greco, Francesco
Publication Year: 2025
Collection: Scuola Universitaria Superiore Pisa Sant'Anna: CINECA IRIS
Subject Terms: almond shell waste; bioderived composite; biomass valorization; laser-induced graphene; sensors
Description: Laser-induced graphene (LIG) is a 3D conductive carbon material typically produced from petroleum-based polymers via a one-step laser-induced pyrolysis in air, without chemicals. Recently, the focus has shifted toward bioderived and biodegradable precursors as potentially sustainable alternatives. Here, this approach is advanced by repurposing almond shells–an abundant raw agricultural by-product–blended with chitosan to form almond shell composites (ASC). ASC exhibits over 60% weight loss after 90 days under soil burial. It serves both as a bioderived substrate for electronics and as a precursor for LIG. ASC is converted into LIG through UV and IR laser scribing, and its structure is thoroughly investigated. ASC-LIG achieves sheet resistance values as low as 114.3 ± 0.9 Ω sq−1 (UV), and an electrochemical impedance modulus |Z| ≈ 1 kΩ at 106 Hz (1 cm2 electrodes). It is implemented in proof-of-concept electronic devices, including circuits with resistive and capacitive elements, and humidity sensors, which show sensitivities of 2.25 ± 0.13 pf%RH−1 (30%–55% RH) and 19.8 ± 2.69 pf%RH−1 (55%–80% RH). These results highlight the potential of upcycling agricultural by-products into functional materials, demonstrating the suitability of ASC-LIG for transient electronic applications such as environmental sensors.
Document Type: article in journal/newspaper
Language: English
Relation: info:eu-repo/semantics/altIdentifier/wos/001523637000001; numberofpages:15; journal:ADVANCED FUNCTIONAL MATERIALS; https://hdl.handle.net/11382/580792
DOI: 10.1002/adfm.202507462
Availability: https://hdl.handle.net/11382/580792; https://doi.org/10.1002/adfm.202507462; https://advanced.onlinelibrary.wiley.com/doi/10.1002/adfm.202507462
Rights: info:eu-repo/semantics/openAccess
Accession Number: edsbas.96413420
Database: BASE