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Direct routes to functional RAFT agents from substituted N-alkyl maleimides

Title: Direct routes to functional RAFT agents from substituted N-alkyl maleimides
Authors: Rosa Catania; Ruggero Foralosso; Lampros Spanos; Emanuele Russo; Francesca Mastrotto; Pratik Gurnani; Kevin Butler; Huw Williams; Snow Stolnik; Giuseppe Mantovani
Contributors: Catania, Rosa; Foralosso, Ruggero; Spanos, Lampro; Russo, Emanuele; Mastrotto, Francesca; Gurnani, Pratik; Butler, Kevin; Williams, Huw; Stolnik, Snow; Mantovani, Giuseppe
Publication Year: 2022
Collection: Padua Research Archive (IRIS - Università degli Studi di Padova)
Description: N-substituted maleimides have become an indispensable tool for the synthesis of bioconjugates and functional materials. Herein, we present three strategies for the incorporation of N-alkyl substituted maleimides into RAFT agents and show that these maleimide-derived CTAs can be used to easily introduce a range of chemical functionality at the β-position of polymer chains, resulting in α,β,ω-functional RAFT polymers. With both functional maleimides and RAFT agents that are increasingly available on the market, the approach presented in this study could facilitate the synthesis of end-functional macromolecules and will complement well the range of existing synthetic routes, including those utilising N-substituted maleimides, to functional polymeric materials.
Document Type: article in journal/newspaper
File Description: ELETTRONICO
Language: English
Relation: info:eu-repo/semantics/altIdentifier/wos/WOS:000885061600001; volume:13; issue:45; firstpage:6261; lastpage:6267; numberofpages:7; journal:POLYMER CHEMISTRY; https://hdl.handle.net/11577/3461171
DOI: 10.1039/d1py01565f
Availability: https://hdl.handle.net/11577/3461171; https://doi.org/10.1039/d1py01565f
Rights: info:eu-repo/semantics/openAccess ; license:Creative commons ; license uri:http://creativecommons.org/licenses/by/4.0/
Accession Number: edsbas.96FAA50A
Database: BASE