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Hybrid direct ink writing of silicone-based emulsions for advanced Biosilicate® scaffolds

Title: Hybrid direct ink writing of silicone-based emulsions for advanced Biosilicate® scaffolds
Authors: Diamanti V.; Elsayed H.; Bernardo E.
Contributors: Diamanti, V.; Elsayed, H.; Bernardo, E.
Publisher Information: Elsevier Ltd
Publication Year: 2026
Collection: Padua Research Archive (IRIS - Università degli Studi di Padova)
Subject Terms: Direct Ink Writing; Emulsion; Infiltration; Photopolymerization; Polymer-derived-ceramics
Description: Preceramic polymer emulsions have recently shown great potential in the production of ceramics featuring a glassy matrix owing to their ability to achieve a high degree of homogenization of fillers, here introduced as aqueous solutions. The present study seeks to extend this strategy to the class of glass-ceramic materials, specifically targeting the Biosilicate® composition. Silicone blends are successfully developed and combined with Direct Ink Writing and thermal treatment in air to fabricate highly porous biosilicate-like scaffolds (up to 94 % total porosity) with outstanding strength-to-density ratios. Firing under nitrogen atmosphere is also explored focusing on its effects on the crystalline phase assemblage, morphology, and physical properties of the scaffolds. Lastly, two post-processing strategies, involving bioresin coating and infiltration respectively, are investigated to mechanically reinforce the air-synthesized polymer-derived scaffolds.
Document Type: article in journal/newspaper
Language: English
Relation: info:eu-repo/semantics/altIdentifier/wos/WOS:001652571000001; volume:46; issue:7; journal:JOURNAL OF THE EUROPEAN CERAMIC SOCIETY; https://hdl.handle.net/11577/3574667
DOI: 10.1016/j.jeurceramsoc.2025.118105
Availability: https://hdl.handle.net/11577/3574667; https://doi.org/10.1016/j.jeurceramsoc.2025.118105
Rights: info:eu-repo/semantics/openAccess ; license:Creative commons ; license uri:http://creativecommons.org/licenses/by/4.0/
Accession Number: edsbas.A22F2DDC
Database: BASE