| Title: |
A holistic review on the direct recycling of lithium-ion batteries from electrolytes to electrodes |
| Authors: |
Hayagan, Neil; Aymonier, Cyril; Croguennec, Laurence; Morcrette, Mathieu; Dedryvère, Rémi; Olchowka, Jacob; Philippot, Gilles |
| Contributors: |
Institut de Chimie de la Matière Condensée de Bordeaux (ICMCB); Université de Bordeaux (UB)-Institut Polytechnique de Bordeaux-Institut de Chimie - CNRS Chimie (INC-CNRS)-Centre National de la Recherche Scientifique (CNRS); Laboratoire de Réactivité et de Chimie des Solides - UMR CNRS 7314 UPJV (LRCS); Advanced Lithium Energy Storage Systems - ALISTORE-ERI (ALISTORE-ERI); Institut de Chimie - CNRS Chimie (INC-CNRS)-Centre National de la Recherche Scientifique (CNRS)-Institut de Chimie - CNRS Chimie (INC-CNRS)-Centre National de la Recherche Scientifique (CNRS)-Université de Picardie Jules Verne (UPJV)-Centre National de la Recherche Scientifique (CNRS); Réseau sur le stockage électrochimique de l'énergie (RS2E); Aix Marseille Université (AMU)-Université Toulouse III - Paul Sabatier (UT3); Communauté d'universités et établissements de Toulouse (Comue de Toulouse)-Communauté d'universités et établissements de Toulouse (Comue de Toulouse)-Université de Haute-Alsace (UHA) Mulhouse - Colmar (Université de Haute-Alsace (UHA))-Collège de France (CdF (institution))-Ecole Nationale Supérieure de Chimie de Paris - Chimie ParisTech-PSL (ENSCP); Université Paris Sciences et Lettres (PSL)-Université Paris Sciences et Lettres (PSL)-Université de Pau et des Pays de l'Adour (UPPA)-Institut de Chimie - CNRS Chimie (INC-CNRS)-Sorbonne Université (SU)-Centre National de la Recherche Scientifique (CNRS)-Institut National Polytechnique (Toulouse) (Toulouse INP); Communauté d'universités et établissements de Toulouse (Comue de Toulouse)-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP); Université Grenoble Alpes (UGA)-Université Grenoble Alpes (UGA)-Nantes Université (Nantes Univ)-Université de Montpellier (UM)-Ecole Nationale Supérieure de Chimie de Montpellier (ENSCM); Université de Montpellier (UM); Institut de Chimie - CNRS Chimie (INC-CNRS)-Centre National de la Recherche Scientifique (CNRS); Institut des sciences analytiques et de physico-chimie pour l'environnement et les materiaux (IPREM); Université de Pau et des Pays de l'Adour (UPPA)-Institut de Chimie - CNRS Chimie (INC-CNRS)-Centre National de la Recherche Scientifique (CNRS); As part of the DESTINY PhD Programme, the authors acknowledge the funding from the European Union's Horizon 2020 research and innovation programme under the Marie Skłodowska-Curie Actions COFUND (Grant Agreement #945357), co-funded by Region Nouvelle Aquitaine (Project Region AAPR2021A-2020-11998810), and from ANR through the STORE-EX Labex project ANR-10-LABX-76-01. This study also received financial support from the French government in the framework of the University of Bordeaux's IdEx “Investments for the Future” program/GPR PPM. We also acknowledge the CNRS.; ANR-10-LABX-0076,STORE-EX,Laboratory of excellency for electrochemical energy storage(2010) |
| Source: |
ISSN: 2050-7488. |
| Publisher Information: |
CCSD; Royal Society of Chemistry |
| Publication Year: |
2024 |
| Collection: |
Université Toulouse III - Paul Sabatier: HAL-UPS |
| Subject Terms: |
Circular economy; Hydrometallurgy; Pyrometallurgy; Recycling; [CHIM.MATE]Chemical Sciences/Material chemistry; [CHIM.ANAL]Chemical Sciences/Analytical chemistry; [CHIM.POLY]Chemical Sciences/Polymers; [CHIM.THEO]Chemical Sciences/Theoretical and/or physical chemistry |
| Description: |
International audience ; Lithium-ion batteries (LIBs) present a global challenge in managing their end-of-life (EOL) issues. As LIB's raw materials are critical and valuable, they are considered as a secondary resource. The volume of publications and patents on LIB recycling has significantly increased, rising a 32% annual growth, compared to a 4% increase in all scientific chemical literature within a decade, reflecting the emergence of this research topic. In a circular economy context, achieving high recycling efficiency of all LIB components and reusing recycled raw materials for battery production are essential. The increase in recycling efficiency is further promoted by government regulations aiming for carbon neutrality and sustainable society with lower environmental impacts. Conventional and destructive recycling methods, pyrometallurgy and hydrometallurgy, focusing on specific metals are insufficient to achieve these goals. Therefore, this review discusses the emerging topic of direct recycling, which recovers, regenerates, and reuses main battery components: electrolyte as well as negative and positive electrodes to fabricate new LIBs. Although this approach may complicate the process, it significantly increases recovery rates, prevents component destruction, and minimizes losses. This critical review offers ideas and methods to provide new perspectives on recycling the main components of LIBs. |
| Document Type: |
article in journal/newspaper |
| Language: |
English |
| DOI: |
10.1039/d4ta04976d |
| Availability: |
https://univ-pau.hal.science/hal-04801933; https://univ-pau.hal.science/hal-04801933v1/document; https://univ-pau.hal.science/hal-04801933v1/file/HayaganNeil_JMaterChemA_2024.pdf; https://doi.org/10.1039/d4ta04976d |
| Rights: |
https://about.hal.science/hal-authorisation-v1/ ; info:eu-repo/semantics/OpenAccess |
| Accession Number: |
edsbas.AAB7A0CF |
| Database: |
BASE |