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Understanding Ion Rejection Mechanism of Freeze Desalination by Molecular Dynamics Simulation

Title: Understanding Ion Rejection Mechanism of Freeze Desalination by Molecular Dynamics Simulation
Authors: Jannat, Mahbuba
Source: All Graduate Theses and Dissertations, Fall 2023 to Present
Publisher Information: DigitalCommons@USU
Publication Year: 2024
Collection: Utah State University: DigitalCommons@USU
Subject Terms: Freeze Desalination; Ion Rejection; MD Simulations; Molecular Dynamics Simulations; Desalination; Free energy; Diffusion; Mechanical Engineering
Description: This study explores a method called freeze desalination, which uses the natural process of ice formation to remove salt from water at lower than freezing temperature of water, which is 235K (Freezing temperature of this water model is 249K), making it safe for potable water. Unlike traditional methods, freeze desalination can be more efficient and environmentally friendly, but how it rejects salt at the molecular level is not very clear to understand. Using molecular dynamics simulation, this research aims to uncover the details of this process. We focused on understanding how water molecules interact with salt ions during freezing. Our findings showed that over 90% of salt ions can be successfully removed from the water under optimal conditions, with certain temperatures and settings leading to the best results. Specifically, we found that sodium ions are removed more effectively than chloride ions. This difference is due to how sodium and chloride ions interact with the surrounding water molecules, which was measure by calculation of free energies. These insights are crucial for improving the technique and making it a viable option for purifying water in different settings. Overall, this work provides a clearer picture of how freeze desalination works at a microscopic level, offering guidance on how to optimize this process for better performance. This could have significant implications for water purification technology, potentially leading to more widespread use of freeze desalination in the future.
Document Type: text
File Description: application/pdf
Language: unknown
Relation: https://digitalcommons.usu.edu/etd2023/268; https://digitalcommons.usu.edu/context/etd2023/article/1257/viewcontent/MAEetd2024Aug_Jannat_Mahbuba.pdf
DOI: 10.26076/5efc-f077
Availability: https://digitalcommons.usu.edu/etd2023/268; https://doi.org/10.26076/5efc-f077; https://digitalcommons.usu.edu/context/etd2023/article/1257/viewcontent/MAEetd2024Aug_Jannat_Mahbuba.pdf
Rights: Copyright for this work is held by the author. Transmission or reproduction of materials protected by copyright beyond that allowed by fair use requires the written permission of the copyright owners. Works not in the public domain cannot be commercially exploited without permission of the copyright owner. Responsibility for any use rests exclusively with the user. For more information contact digitalcommons@usu.edu.
Accession Number: edsbas.BF88A54A
Database: BASE