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A machine vision tool for facilitating the optimization of large-area perovskite photovoltaics

Title: A machine vision tool for facilitating the optimization of large-area perovskite photovoltaics
Authors: Nina Taherimakhsousi; Mathilde Fievez; Benjamin P. MacLeod; Edward P. Booker; Emmanuelle Fayard; Muriel Matheron; Matthieu Manceau; Stéphane Cros; Solenn Berson; Curtis P. Berlinguette
Source: npj Computational Materials, Vol 7, Iss 1, Pp 1-10 (2021)
Publisher Information: Nature Portfolio
Publication Year: 2021
Collection: Directory of Open Access Journals: DOAJ Articles
Subject Terms: Materials of engineering and construction. Mechanics of materials; TA401-492; Computer software; QA76.75-76.765
Description: We report a fast, reliable and non-destructive method for quantifying the homogeneity of perovskite thin films over large areas using machine vision. We adapt existing machine vision algorithms to spatially quantify multiple perovskite film properties (substrate coverage, film thickness, defect density) with pixel resolution from pictures of 25 cm2 samples. Our machine vision tool—called PerovskiteVision—can be combined with an optical model to predict photovoltaic cell and module current density from the perovskite film thickness. We use the measured film properties and predicted device current density to identify a posteriori the process conditions that simultaneously maximize the device performance and the manufacturing throughput for large-area perovskite deposition using gas-knife assisted slot-die coating. PerovskiteVision thus facilitates the transfer of a new deposition process to large-scale photovoltaic module manufacturing. This work shows how machine vision can accelerate slow characterization steps essential for the multi-objective optimization of thin film deposition processes.
Document Type: article in journal/newspaper
Language: English
Relation: https://doi.org/10.1038/s41524-021-00657-8; https://doaj.org/toc/2057-3960; https://doaj.org/article/93667ca46ddd41e09df0a36ed00798d4
DOI: 10.1038/s41524-021-00657-8
Availability: https://doi.org/10.1038/s41524-021-00657-8; https://doaj.org/article/93667ca46ddd41e09df0a36ed00798d4
Accession Number: edsbas.D2DAD53
Database: BASE