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Overcoming photobleaching in imaging of single barium atoms in a solid xenon matrix

Title: Overcoming photobleaching in imaging of single barium atoms in a solid xenon matrix
Authors: M. Yvaine; D. Fairbank; J. Soderstrom; C. Taylor; J. Stanley; T. Walton; C. Chambers; A. Iverson; W. Fairbank; S. Al Kharusi; A. Amy; E. Angelico; A. Anker; I. J. Arnquist; A. Atencio; J. Bane; V. Belov; E. P. Bernard; T. Bhatta; A. Bolotnikov; J. Breslin; P. A. Breur; J. P. Brodsky; E. Brown; T. Brunner; E. Caden; G. F. Cao; D. Cesmecioglu; E. Chambers; B. Chana; D. Chernyak; M. Chiu; R. Collister; M. Cvitan; T. Daniels; L. Darroch; R. DeVoe; M. L. di Vacri; M. J. Dolinski; B. Eckert; M. Elbeltagi; R. Elmansali; N. Fatemighomi; B. Foust; Y. S. Fu; D. Gallacher; N. Gallice; G. Giacomini; W. Gillis; C. Gingras; R. Gornea; G. Gratta; C. A. Hardy; S. Hedges; E. Hein; J. D. Holt; E. W. Hoppe; A. Karelin; D. Keblbeck; I. Kotov; A. Kuchenkov; K. S. Kumar; A. A. Kwiatkowski; A. Larson; M. B. Latif; K. G. Leach; A. Lennarz; D. S. Leonard; H. Lewis; G. Li; Z. Li; C. Licciardi; R. Lindsay; R. MacLellan; S. Majidi; C. Malbrunot; J. Masbou; K. McMichael; M. Medina Peregrina; M. Moe; B. Mong; D. C. Moore; C. R. Natzke; X. E. Ngwadla; K. Ni; A. Nolan; S. C. Nowicki; J. C. Nzobadila Ondze; A. Odian; J. L. Orrell; G. S. Ortega; C. T. Overman; L. Pagani; H. Peltz Smalley; A. Perna; A. Pocar; V. Radeka; E. Raguzin; H. Rasiwala; D. Ray; S. Rescia; G. Richardson; R. Ross; P. C. Rowson; R. Saldanha; S. Sangiorgio; S. Schwartz; S. Sekula; L. Si; A. K. Soma; F. Spadoni; V. Stekhanov; X. L. Sun; S. Thibado; A. Tidball; T. Totev; S. Triambak; T. Tsang; O. A. Tyuka; E. van Bruggen; M. Vidal; M. Walent; K. Wamba; H. W. Wang; Q. D. Wang; W. Wang; Y. G. Wang; M. Watts; M. Wehrfritz; L. J. Wen; U. Wichoski; S. Wilde; M. Worcester; H. Xu; L. Yang; M. Yu; O. Zeldovich
Source: Physical Review Research, Vol 6, Iss 4, p 043193 (2024)
Publisher Information: American Physical Society
Publication Year: 2024
Collection: Directory of Open Access Journals: DOAJ Articles
Subject Terms: Physics; QC1-999
Description: Neutrinoless double beta decay is one of the most sensitive probes for new physics beyond the Standard Model of particle physics. One of the isotopes under investigation is ^{136}Xe, which would double beta decay into ^{136}Ba. Detecting the single ^{136}Ba daughter provides a sort of ultimate tool in the discrimination against backgrounds. Previous work demonstrated the ability to perform single atom imaging of Ba atoms in a single-vacancy site of a solid xenon matrix. In this paper, the effort to identify signal from individual barium atoms is extended to Ba atoms in a hexa-vacancy site in the matrix and is achieved despite increased photobleaching in this site. Abrupt fluorescence turn-off of a single Ba atom is also observed. Significant recovery of fluorescence signal lost through photobleaching is demonstrated upon annealing of Ba deposits in the Xe ice. Following annealing, it is observed that Ba atoms in the hexa-vacancy site exhibit antibleaching while Ba atoms in the tetra-vacancy site exhibit bleaching. This may be evidence for a matrix site transfer upon laser excitation. Our findings offer a path of continued research toward tagging of Ba daughters in all significant sites in solid xenon.
Document Type: article in journal/newspaper
Language: English
Relation: http://doi.org/10.1103/PhysRevResearch.6.043193; https://doaj.org/toc/2643-1564; https://doaj.org/article/5646cacf213c4ac2a5455b09cebbfb1d
DOI: 10.1103/PhysRevResearch.6.043193
Availability: https://doi.org/10.1103/PhysRevResearch.6.043193; https://doaj.org/article/5646cacf213c4ac2a5455b09cebbfb1d
Accession Number: edsbas.D8C7F4A8
Database: BASE