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Unveiling the quasiparticle behaviour in the pressure-induced high-Tc phase of an iron-chalcogenide superconductor

Title: Unveiling the quasiparticle behaviour in the pressure-induced high-Tc phase of an iron-chalcogenide superconductor
Authors: Zajicek, Zachary; Reiss, Pascal; Graf, David; Prentice, Joseph; Sadki, Y.; Haghighirad, A.A.; Coldea, Amalia
Source: Zajicek, Z, Reiss, P, Graf, D, Prentice, J, Sadki, Y, Haghighirad, A A & Coldea, A 2024, 'Unveiling the quasiparticle behaviour in the pressure-induced high-Tc phase of an iron-chalcogenide superconductor', npj Quantum Materials. https://doi.org/10.1038/s41535-024-00663-1
Publication Year: 2024
Collection: The University of Manchester: Research Explorer - Publications
Description: Superconductivity of iron chalocogenides is strongly enhanced under applied pressure yet its underlying pairing mechanism remains elusive. Here, we present a quantum oscillations study up to 45 T in the high-Tc phase of tetragonal FeSe0.82S.18 up to 22 kbar. Under applied pressure, the quasi-two-dimensional multi-band Fermi surface expands and the effective masses remain large, whereas the superconductivity displays a threefold enhancement. Comparing with chemical pressure tuning of FeSe1−xSx, the Fermi surface expands in a similar manner but the effective masses and Tc are suppressed. These differences may be attributed to the changes in the density of states influenced by the chalcogen height, which could promote stronger spin fluctuations pairing under pressure. Furthermore, our study also reveals unusual scattering and broadening of superconducting transitions in the high-pressure phase, indicating the presence of a complex pairing mechanism.
Document Type: article in journal/newspaper
Language: English
ISSN: 2397-4648
Relation: info:eu-repo/semantics/altIdentifier/pissn/2397-4648
DOI: 10.1038/s41535-024-00663-1
Availability: https://research.manchester.ac.uk/en/publications/6d689a1e-8dba-4113-acd1-0cd87e3c6fa1; https://doi.org/10.1038/s41535-024-00663-1
Rights: info:eu-repo/semantics/openAccess
Accession Number: edsbas.E3D9E812
Database: BASE