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Eco-conscious electromagnetic interference shielding: Mechanically robust, flexible, and recyclable PVA/Graphene composite films for next-generation applications

Title: Eco-conscious electromagnetic interference shielding: Mechanically robust, flexible, and recyclable PVA/Graphene composite films for next-generation applications
Authors: Lekshmi Omana; Reenu Elizabeth John; Deepti Das Krishna; Immanuvel Paul; Runcy Wilson; Justin George; Bejoy Francis; Nellipparambil Viswambharan Unnikrishnan; Kalapurackal Cheriyan George; Rejo Mathew Joseph; Issac Paul; Anoop Chandran
Source: Next Materials, Vol 9, Iss , Pp 101077- (2025)
Publisher Information: Elsevier, 2025.
Publication Year: 2025
Collection: LCC:Technology
Subject Terms: Polyvinyl alcohol; Graphene; Sodium dodecyl sulphate; EMI shielding; Solution casting; Technology
Description: Recyclable and flexible electromagnetic interference (EMI) shielding materials are pivotal for sustainable electronics. This study investigates polyvinyl alcohol (PVA)-graphene-sodium dodecyl sulphate (SDS) nanocomposites synthesized via solution casting, achieving an optimized balance of mechanical strength, shielding efficiency, and recyclability. Microstructural analyses (Raman imaging, SEM, μ-CT) confirmed uniform filler dispersion, while FTIR, XRD, and Raman spectroscopy validated structural integration. TGA demonstrated enhanced thermal stability, alongside significant improvements in flexibility and tensile strength due to graphene incorporation. Frequency-dependent AC conductivity at various temperatures was modelled using the random free energy barrier approach, while electrical conductivity variation with filler concentration adhered to a sigmoidal model. Achieving a remarkable specific shielding efficiency per thickness (SSE/t) of 224.83 dBcm2/g, these composites also exhibit water solubility, supporting their recyclability. Thus, PVA/graphene films emerge as promising candidates for eco-friendly, high-performance EMI shielding solutions.
Document Type: article
File Description: electronic resource
Language: English
ISSN: 2949-8228
Relation: http://www.sciencedirect.com/science/article/pii/S2949822825005957; https://doaj.org/toc/2949-8228
DOI: 10.1016/j.nxmate.2025.101077
Access URL: https://doaj.org/article/fe708bbcebab4bb4868a9dfd5ceaa2ae
Accession Number: edsdoj.fe708bbcebab4bb4868a9dfd5ceaa2ae
Database: Directory of Open Access Journals